Vibrational properties of Ba , _ , K , BiO , A molecular dynamics study

نویسنده

  • P. A. Deymier
چکیده

We present a rigid-ion model of Ba, zK,BiO, for compositions x = 0.25 and x = 0.40. Partial vibrational density ot states of ions in the compounds Ba,, ,? K,, ,,BiO, and Ba,, (,Ki, ,BiO, are reported at room temperature and 100 K. The oxygen modes dominate the vibrational spectrum from 150 up to 82Ocm ‘. The low frequency modes arc associated with the cations. The number of substituted K around an oxygen favors high frequency vibrational modes. Qualitative agreement between the calculated phonon density of states of Ba,, ,, K,, ,BiO, and available experimental data is achieved.

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تاریخ انتشار 2002